Spin-phonon interaction and mode softening in NiF2
Магнетизм
DOI (Low Temperature Physics):
https://doi.org/10.1063/1.1496657Ключові слова:
PACS: 78.30.Hv, 75.50.Ee, 63.20.Dj, 63.20.KrАнотація
The temperature dependence of the four Raman-active phonons in NiF2 has been investigated at temperatures above and below the antiferromagnetic ordering temperature of TN=73 K. All four modes exhibit distinct anomalies in their intensities and frequencies near TN due to spin-phonon coupling. The phonon linewidths also exhibit weak anomalies. From the temperature dependences of the phonon frequencies, estimates are made of the spin-phonon coupling coefficients. The B1g phonon exhibits anomalous mode softening with decreasing temperature from 300 K to TN .Завантаження
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